Chemistry Letters p. 831 - 834 (1981)
Update date:2022-08-15
Topics:
Mori, Toshiaki
Masuda, Hiroyuki
Imai, Hisao
Miyamoto, Akira
Baba, Shigeo
Murakami, Yuichi
A hydrogen-deuterium inverse isotope effect was found for the C-O bond dissociation process in the methanation of adsorbed CO on a Ni catalyst using a pulse technique; the average value of kH/kD was 0.75.Such an effect (0.77) was also found for the steady-state reaction of the CO methanation.It was shown that the adsorbed CO molecule is partially hydrogenated before the C-O bond dissociation.
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