Electrochemistry of THORIUM FLUORIDE (cas 13709-59-6) in LiCl-KCl eutectic melts and methodology for speciation studies with fluorides ions
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Add time:09/10/2019 Source:sciencedirect.com
This paper reports the electrochemical behavior of ThF4 in LiCl-KCl molten salt. It proposes a potentiometric method to determine the complexation constants of thorium (IV) with fluorides. The knowledge of these constants leads to calculate the speciation diagram of Th(IV) species as a function of the concentration of fluoride ions in the salt. These results were extrapolate to give an estimation of the activity coefficient of ThF4 in the molten salt LiF-ThF4 (77.5-22.5 mol%). This salt is retained for the molten salt fast reactor system, currently studied as a Generation IV concept in the domain of nuclear energy.
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