Journal of the American Chemical Society p. 12548 - 12551 (2014)
Update date:2022-08-05
Topics:
Oldenhuis, Nathan J.
Dong, Vy M.
Guan, Zhibin
A commercially available ruthenium(II) PNP-type pincer catalyst (Ru-Macho) promotes the formation of α-chiral tert-butanesulfinylamines from racemic secondary alcohols and Ellmans chiral tert-butanesulfinamide via a hydrogen borrowing strategy. The formation of α-chiral tert-butanesulfinylamines occurs in yields ranging from 31% to 89% with most examples giving >95:5 dr.
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Doi:10.1021/jo00001a048
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