Tetrahedron Letters p. 6023 - 6026 (1997)
Update date:2022-07-29
Topics:
Konno, Hiroyuki
Hiroya, Kou
Ogasawara, Kunio
A meso-1,4-enediol bis-silyl ether 2 having bicyclo[2.2.1]heptene background has been transformed diastereo- and enantioselectively into (-)malyngolide 1, an antibiotic isolated from the blue-green marine algae, Lyngbya majuscula, via Rh(I)-(R)BINAP-catalyzed asymmetrization and diastereoselective modification of the optically active product thus obtained.
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