Dalton Transactions
Paper
the complex and their magnetic moment vectors, canting KAKENHI Grant Number 16K05942. X-ray structure analyses
occurs due to a competition between antiparallel alignments and magnetic experiments were conducted at the Institute of
that cause antiferromagnetic interactions, and the anisotropies Molecular Science, supported by the Nanotechnology Platform
of the Co(II) ions. As a result, a small net magnetisation occurs Program (Molecule and Material Synthesis) of the Ministry of
in the coordination sheet toward the b axis, as shown in Education, Culture, Sports, Science and Technology (MEXT),
Fig. 5(a). Hence, each coordination sheet is spontaneously Japan. Neutron diffraction experiments were performed using
magnetised toward the b axis, and magnetisation cancels out SENJU under the trial use program (2016A0016) of J-PARC and
in the intersheets (Fig. 5(b)). It is likely that weak antiferro- CROSS.
magnetic interactions occur between the sheets via the hydro-
gen bonds.15 The magnetisation in each sheet of this material
is oriented toward the magnetic field below the critical field of
22 600 Oe (Fig. 5(c)). As shown in Fig. 2(c), a rapid increase of
References
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which is consistent with the observed rapid increase; the
assumption shown in Fig. 5 is supported by this value. The
magnetisation increases with the increasing magnetic field
above the critical magnetic field because the canting angle
increases.
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Conclusions
We carried out magnetic, thermal, and neutron diffraction
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Conflicts of interest
There are no conflicts to declare.
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Acknowledgements
This study was partially supported by a Grant from the Faculty
of Science and Technology, Seikei University, and by JSPS
This journal is © The Royal Society of Chemistry 2019
Dalton Trans., 2019, 48, 333–338 | 337