Synthesis p. 3126 - 3136 (2021)
Update date:2022-08-11
Topics:
Kona, Chandrababu Naidu
Oku, Rikuto
Nishii, Yuji
Miura, Masahiro
An iridium-catalyzed acylmethylation and a rhodium-catalyzed amidation of naphthalene derivatives are reported, adopting sulfoxonium ylides and dioxazolones as carbene and nitrene transfer agents, respectively. The use of SMe group as a directing group was key to ensure the peri -selective functionalization, and it can be easily removed or diversely transformed to other synthetically useful functionalities after the catalysis.
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