Journal of the Chemical Society, Faraday Transactions 1: Physical Chemistry in Condensed Phases p. 1937 - 1942 (1982)
Update date:2022-08-10
Topics:
Caldin, Edward
Field, John P.
The kinetics of the formation of the electron donor-acceptor complex between iodine and imidazole in 1-chlorobutane at -64 deg C have been investigated by an improved microwave temperature-jump apparatus.The forward rate constant kf is (3.3+/-0.4)x1E9 dm3 mol-1 s-1.This is nearly the same as the diffusion-controlled value kD calculated from the simple Smoluchowsky model for reaction at every encounter between spherical molecules, without geometrical requirements, in a homogeneous fluid (kf/kD=0.8).
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