Organic Letters p. 1260 - 1263 (2010)
Update date:2022-07-30
Topics:
Smith III, Amos B.
Tong, Rongbiao
Chemical Equation Presented A new class of bifunctional linchpins bearing electrophilic sites β or γ to a silyl group have been designed, synthesized, and demonstrated to be competent In tricomponent unions exploiting Type II Anion Relay Chemistry (ARC). High diastereoselectivities were observed when a phenyl moiety (R2) served as an anion-stabilizing group (ASG) adjacent to a methyl susbtituent (R 1), while diastereomeric mixtures were obtained when a phenylthiol moiety served as the ASG, irrespective of α-substitution.
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