Angewandte Chemie - International Edition p. 1241 - 1244 (2006)
Update date:2022-09-26
Topics:
Shaver, Michael P.
Allan, Laura E. N.
Rzepa, Henry S.
Gibson, Vernon C.
The mechanism of styrene polymerization by α-diimine iron complexes correlates with the metal spin state of the catalyst. Experimental and theoretical studies indicate that high-spin catalysts are halogenophilic, resulting in atom transfer radical polymerization (ATRP), while intermediate-spin complexes are carbophilic giving rise to catalytic chain transfer (CCT, see graph). (Graph Presented)
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(1981)
