Synlett p. 725 - 727 (1997)
Update date:2022-08-11
Topics:
Allin, Steven M.
Button, Martin A. C.
Shuttleworth, Stephen J.
Thermally induced [3,3]-sigmatropic rearrangement of 3-amino-1,5-diene substrates occurs to give the corresponding enamine products in high yield and with excellent trans:cis enamine selectivity. The enamine produced during the amino-Cope rearrangement has been directly derivatized, representing the first report of a tandem amino-Cope rearrangemenl/enamine alkylation reaction. The potential of this novel synthetic strategy is outlined.
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