Tetrahedron Letters p. 7665 - 7668 (1997)
Update date:2022-08-11
Topics:
Greer, Melinda L.
Duncan, Joseph R.
Duff, Janice L.
Blackstock, Silas C.
2,3-Dimethylquinoxaline-N,N'-dioxide (DMQDO) and phenazine-N,N'-dioxide (PDO) bind to tetracyanoethylene (TCNE) in solution, with complexation constants of 4.8(7) and 1.2(7) M-1, respectively in CH2Cl2. Crystallization of the mixtures affords two-component solids which contain weakly bound one-dimensional donor-acceptor arrays. The DA interactions create DA ladder domains in the (DMQDO)2TCNE solid and single-stranded DA chains in the (PDO)TCNE crystal.
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