Chemical Physics Letters p. 411 - 418 (1995)
Update date:2022-08-11
Topics:
Keita, Bineta
Essaadi, Khalid
Nadjo, Louis
Desmadril, Michel
The kinetics of NADH oxidation by 3 Dawson-type mixed heteropolyanions were studied in buffered aqueous pH = 7 medium, by the stopped flow technique and UV-visible spectroscopy.The log of k was a linear function of the E0 of the first redox systems of the heteropolyanions with a slope of 16.5 V-1.The results indicate that, in the present case, the oxidation of NADH proceeds by a multistep mechanism involving initial rate-limiting one-electron transfer.An estimate of the E0 value for the one-electron NADH/NADHcation radical couple has been obtained.
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