A new highly active polymer supported ruthenium nanocatalyst for the hydrolytic dehydrogenation of Dimethylamine (cas 124-40-3)-borane

Add time:09/24/2019    Source:sciencedirect.com

Herein, we report a highly active [email protected] nanocatalyst for the hydrolytic dehydrogenation of dimethylamine-borane under room conditions. The [email protected] nanocatalyst was readily prepared, stabilized and used effectively in the catalytic dehydrogenation reaction of dimethylamine-borane in water at room conditions. The prepared [email protected] nanocatalyst was characterized using advanced analytical methods such as XPS, XRD, HR-TEM, etc. The characterization analyzes shown that Ru metals are uniformly distributed on the PVP support surface; the mean particle of catalyst size was found to be 2.78 ± 0.16 nm. The catalytic test showed that DMAB had a high catalytic activity with [email protected] in aqueous solutions, and TOF value was found to be 2500.52 h−1 for hydrolytic dehydrogenation of DMAB at room conditions. The study also included kinetic data such as activation parameters for different temperatures, catalyst concentration, and substrate concentration experiments.

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