Tetrahedron Letters p. 145 - 148 (1996)
Update date:2022-08-03
Topics:
Wee, Andrew G.H.
Liu, Baosheng
The Rh2(OAc)4-catalysed C-H insertion in chiral ester diazoanilides was investigated and was found to yield 4-substituted 2-pyrrolidinones with moderate to high e.e. (37-98%) after decarbalkoxylation. Electronic effects were found to oppose steric effects in influencing the enantioselectivity of the reaction in N-arylethyl diazoanilides.
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