Journal of the Chemical Society, Dalton Transactions p. 3375 - 3381 (1990)
Update date:2022-08-05
Topics:
Okuno, Hiroaki (Yohmei)
Uoto, Kouichi
Tomohiro, Takenori
Youinou, Marie-Therese
A new type of active-site analogues for 4Fe-4S iron-sulphur proteins is introduced, where the active site core is surrounded by an intramolecular hydrophobic domain formed by a 36-membered ring consisting of a methylene backbone.An efficient synthesis of the macrocyclic ligands 1,10,19,28-tetra(4-mercaptobenzoyl)-1,10,19,28-tetra-azacyclohexatriacontane and 1,10,19,28-<4-(mercaptomethyl)benzoyl>-1,10,19,28-tetra-azacyclohexatriacontane and 1,10,19,28-tetra-(3-mercapto-3-methylbutanoyl)-1,10,19,28-tetra-azacyclohexatriacontane is described.Their reaction with
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