Transactions of the Faraday Society p. 2930 - 2940 (1969)
Update date:2022-08-29
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DONOVAN RJ
HUSAIN D
JACKSON PT
The primary processes occurring in the photolysis of SOCl//2 have been examined by use of kinetic absorption spectroscopy in the ultraviolet and vacuum ultraviolet. Photodissociation involves the fission of one sulfurchlorine bond, leaving an energized SOCl radical which may then undergo unimolecular decomposition to yield an SO radical and a further chlorine atom, or is stabilized by collision. The kinetics of the SO radical so formed are examined and a mechanism for removal is proposed. Two new electronic states of the SO radical are identified via new absorption systems in the vacuum ultraviolet.
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