Bulletin of the Chemical Society of Japan p. 909 - 913 (1983)
Update date:2022-08-16
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Gas-phase benzene oxychlorination was carried out over a CuCl//2-CeCl//3/Al//2O//3 catalyst. A kinetic model is proposed which permits us to obtain a rate equation capable of reproducing experimental results. The presence of cerium in the catalyst increases the reaction rate and maintains the conversion level for a long time. It seems that this element facilitates copper reoxidation by making the total rate independent of the partial pressure of oxygen and stabilizes the active phase of the catalyst.
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