Journal of the American Chemical Society p. 2180 - 2186 (1989)
Update date:2022-08-17
Topics:
Gaillard, Elizabeth
Fox, Marye Anne
Wan, Peter
Excitation of 9-fluorenol in methanol and methanol-water mixtures leads to both heterolytic and homolytic cleavage via the singlet excited state.The partitioning between homolysis and heterolysis is controlled by solvent composition, the rate constant for cation formation being a function of the solvent dielectric constant.The rate constants of intersystem crossing, fluorescence, and singlet-derived radical formation are linear functions of the mole fraction of water.
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