Chemical Physics Letters p. 267 - 273 (1996)
Update date:2022-08-16
Topics:
Ananchenko, G. S.
Bagryanskaya, E. G.
Tarasov, V. F.
Sagdeev, R. Z.
Paul, H.
31P stimulated nuclear polarization spectra and their dependence on time after photolysis of (2,4,6-trimethylbenzoyl)diphenylphosphine oxide in micellar solution of sodium octyl- (SOS) and dodecylsulfate (SDS) are investigated and discussed in terms of the numerical solution of the stochastic Liouville equation for a microreactor model.The decay of the geminate radical pair is found to be about 2.5 times slower in SDS than in the SOS micelles due to a larger re-encounter rate in the latter one.Simulation of the experimental results further suggests J0= ca. -1.6*1010 rad/s for the exchange interaction at contact distance, and an increasing micellar size with increasing radical size.
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