Journal of Physical Chemistry p. 5529 - 5532 (1991)
Update date:2022-08-31
Topics:
Braun, Charles L.
Smirnov, Sergei N.
Brown, Steven S.
Scott, T. W.
Durene (1,2,4,5-tetramethylbenzene) dissolved in n-hexane was photoionized by 35-ps light pulses at 266 nm.Transient absorption at 1064 nm arising chiefly from geminate electrons was detected and used to monitor the recombination of the electron-cation pairs produced by two-photon ionization.An excellent fit to the recombination kinetics at 208 K was obtained by assuming that the distribution of initial electron-cation separations was of the form r2EXP=r2/(2L3)exp(-r/L) with a mean radius 3L = 5.7 nm.
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