Journal of Organometallic Chemistry p. C26 - C30 (1990)
Update date:2022-08-11
Topics:
Cambie, Richard C.
Metzler, Michael R.
Rutledge, Peter S.
Woodgate, Paul D.
Orthomanganated complexes have been made from carbonyl derivatives of the ring-C aromatic diterpenoids podocarpic acid and dehydroabietic acid.Activation of these complexes with Me3NO followed by coupling reactions with various substituted alkenes results in efficient substitution at C14.In some cases a tetracyclic indenol derivative is formed directly.Insertion of an alkyne also leads to cyclopentaannulation.
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