Tetrahedron Letters p. 5033 - 5036 (1980)
Update date:2022-08-11
Topics:
Kojima, Yasuhiro
Kato, Natsuki
In order to elucidate the structure-activity relationships of the antifeeding diterpenes having a neo-clerodane skeleton, clerodin homolog 5 was stereoselectively synthetized through 18 steps via a key intermediate 11.Perhydrofuro<2,3-b>furan ring in the synthesized homolog was more unstable than that of the natural product, and gave a tri-MeOH adduct 3 in a similar behavior to that of the model compound 1 and 2.
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