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Plots of observed rate of pseudo-first-order decay, kobs, versus concentration of tetrabutylammonium acetate for deprotonation of the radical cations of (open circles) N,N-dimethylaniline, 1c, and N,N,-dimethylaniline with (filled circles) a 4-methyl subs
Brønsted plot of the logarithm of the bimolecular rate constant for deprotonation of the radical cations of N,N-dimethylaniline derivatives: (closed circles) 4-substituted-N,N-dimethylanilines, 1a-1e; (open circle) N,N,2-trimethylaniline, 2; (open squares
Structures of Sterically Twisted N,N-Dimethylaniline Radical Cations, and the Dihedral Angles between the Planes Containing the Aromatic Ring and the Amino Nitrogen, θ.
Absorption spectra of the radical cations of (closed circles) N,N-dimethylaniline, 1c, and N,N,-dimethylaniline with (open circles) a 2-methyl substituent, 2, (closed squares) a 2-tert-butyl substituent, 3, and (open squares) 2,6-dimethyl substituents, 4,
Plot of the logarithm of the rate constant for unimolecular deprotonation (log(k-H )) versus the cosine squared of the dihedral angle θ, for the simple dimethylanilines, assumed to be appropriate for the intramolecular deprotonating anilines here.
